* γελῶ (gelō): This verb means "to laugh," but it can also encompass a smile, particularly a light or joyful one. It's probably the closest single word.
* μείδιασμα (meidiasma): This noun refers to a "smile," often a gentle or sweet one.
Other words might be used depending on the type of smile, for instance, a smirk might require a different word altogether. The best choice would depend on the specific literary context.