Here's why:
* Chronicles: The series title itself matches your description.
* Grandfather with Secrets: While not directly a grandfather, the Professor in the books acts as a father figure and hides a secret world of Narnia from the children.
* Moving to a New House: The Pevensie children are evacuated from London during World War II to the Professor's country house.
* Brother and Sister: The story follows four siblings: Peter, Susan, Edmund, and Lucy.
* Boy Found Some "Lit": Edmund finds a magical lamp in Narnia that reveals the world's secrets.
Let me know if this is the book you were thinking of!